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Abstract The Andes of western Argentina record spatiotemporal variations in morphology, basin geometry, and structural style that correspond with changes in crustal inheritance and convergent margin dynamics. Above the modern Pampean flat‐slab subduction segment (27–33°S), retroarc shortening generated a fold‐thrust belt and intraforeland basement uplifts that converge north of ∼29°S, providing opportunities to explore the effects of varied deformation and subduction regimes on synorogenic sedimentation. We integrate new detrital zircon U‐Pb and apatite (U‐Th)/He analyses with sequentially restored, flexurally balanced cross sections and thermokinematic models at ∼28.5–30°S to link deformation with resulting uplift, erosion, and basin accumulation histories. Tectonic subsidence, topographic evolution, and thermochronometric cooling records point to (a) shortening and distal foreland basin accumulation at ∼18–16 Ma, (b) thrust belt migration, changes in sediment provenance, and enhanced flexural subsidence from ∼16 to 9 Ma, (c) intraforeland basement deformation, local flexure, and drainage reorganization at ∼12–7 Ma, and (d) out‐of‐sequence shortening and exhumation of foreland basin fill by ∼8–2 Ma. Thrust belt kinematics and the reactivation of basement heterogeneities strongly controlled tectonic load configurations and subsidence patterns. Geo/thermochronological data and model results resolve increased shortening and combined thrust belt and intraforeland basement loading in response to ridge collision and Neogene shallowing of the subducted oceanic slab. Finally, this study demonstrates the utility of integrated flexural thermokinematic and erosion modeling for evaluating the geometries, rates, and potential drivers of retroarc deformation and foreland basin evolution during changes in subduction. 

Abstract Understanding the effects of flat slab subduction on mountain building, arc magmatism, and basin evolution is fundamental to convergent‐margin tectonics, with implications for potential feedbacks among geodynamic, magmatic, and surface processes. New stratigraphic and geochronological constraints on Cenozoic sedimentation and magmatism in the southern Central Andes of Argentina (31°S) reveal shifts in volcanism, foreland/hinterland basin development, sediment accumulation, and provenance as the retroarc region was structurally partitioned during slab flattening. Detrital zircon U‐Pb age distributions from the western (Calingasta basin), central (Talacasto and Albarracín basins), and eastern (Bermejo foreland basin) segments of the retroarc basin system preserve syndepositional volcanism and orogenic unroofing of multiple tectonic provinces. Initial shortening‐related exhumation of the Principal Cordillera at 24–17 Ma was recorded by the accumulation of distal eolian deposits bearing Oligocene–Eocene zircons from the Andean magmatic arc. The Calingasta basin chronicled volcanism and basement shortening in the Frontal Cordillera at ~17–11 Ma, as marked by an upward coarsening succession of fluvial to alluvial fan deposits with a sustained zircon U‐Pb age component that matches pervasive Permian‐Triassic bedrock in the hinterland. An ~450 km eastward inboard sweep of volcanism at 11 Ma coincided with the inception of flat slab subduction, and subsequent thin‐skinned shortening in the Precordillera fold‐thrust belt that exhumed wedge‐top deposits and induced cratonward (eastward) advance of flexural subsidence into the Bermejo foreland basin. This foreland basin was structurally partitioned as basement uplifts of the Sierras Pampeanas transformed a fluvial megafan sediment routing network into smaller isolated alluvial fan systems fed by adjacent basement blocks.